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33___PPT10i.JPx+D='  = @B +r#h#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖD[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dl 0<pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#  r#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖD[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dl 0<pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#  r#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖ"D[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dd 0pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#    0 0 M(  T  C ,AIMG_4419m&4  Zjpp9?g  2010t^,{26g  '($|  Bm?$v Ve11g18efgV 15:00 16:40 0WpSN'Yf[irt'Y|i-N212Ye[,,'-d B  H{?J!#  \Characterization at picometres precision of structure and properties of ferroelectric oxides]]-.   >    <3fQ"`3P$4 Photograph by Xiaodong Hu,  Hć3s?"` !%P ,>%fg Yec _VN)R ^xvz-N_Forschungszentrum Jlich GmbH)xvzXT [N'Yf[VE5uN(xvz-N_Yec0E&<>&(P    X  <܋. 0 PT|N: SfN Yec 62767621 huxd@pku.edu.cn 8)'g g@   BL\O"`jC#( bAbstract: Epitaxial thin films of ferroelectric oxides have attracted increasingly intensive research both for fundamental and application issues. The physical properties of these film systems depend strongly on the particular microstructure and configuration of lattice defects. By means of an aberration corrector in a high-resolution transmission electron microscope the value of the spherical aberration CS can be tuned to negative values resulting in a novel imaging technique: The negative CS imaging (NCSI) technique. The images obtained with the NCSI technique are superior to positive CS images in the magnitude of the contrast and the image intensity of atom columns. The image signal obtained with the NCSI technique is significantly more robust against noise, resulting in measurement of atomic positions with a precision of a few picometres. In this talk, we present the results of a study using NCSI technique of the epitaxial thin-film system of PbZr0.2Ti0.8O3. The positions of all the atomic species are measured, unit cell by unit cell, with a precision of a few picometres. On this basis the relative ion displacement and the electric dipole moment for the individual unit cells are calculated. The resulting dipole moments depict the details of polarization domains, domain walls, as well as the local variation of spontaneous polarization at defect areas. vc  Wa   '   O        0nn  B I01 &SN'Yf[irtf[bQZ`irtNPgeirt@b ' ,  <3fQ"`1 3 ,/events/icmp10f.xml,-, 0(J  S ~rkrk ԔԔ8c8c?C#* QZ`irt-SN'Yf[[W2 'X'X ,  T@?\O ?"6?@`NNN?N N 2X _[h 1996t^_-NVyf[birtxvz@bZSXf[MO sNSN'Yf[irtf[bYec0ZSXu[^ Ye萰eN~OyNMb0HQTNN^~'`IQf[0Oo`IQf[T~s|IQP[f[vxvz02007t^_Y;NxvzeT:NhbI{yoCQIQf[ vsQ]\OSh(WPhysical Review Letters0Advanced MaterialsTACS NanoI{VEW TBg_ N04$$nH  0nnH  0+nF ? 33___PPT10i.JPx+D=' = @B +r#}+#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖ"D[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dd 0pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#    0 0 m(  T  C ,AIMG_4419m5%4  Zjpp9?g  2010t^,{26g  '($|  Bm?G Ve11g18efgV 15:00 16:40 0WpSN'Yf[irt'Y|i-N212Ye[,,'-d B  H{?Jp#  \Characterization at picometres precision of structure and properties of ferroelectric oxides]]-.   >    <3fQ"`2#$3 Photograph by Xiaodong Hu,  Hć3s?"`r $& *>%fg Yec _VN)R ^xvz-N_Forschungszentrum Jlich GmbH)xvzXT [N'Yf[VE5uN(xvz-N_Yec.E&B>&(P    F  <܋- / HT|N: O'YOYec emaildpyu@pku.edu.cn .%#g$-@(  BL\O"`&$<( bAbstract: Epitaxial thin films of ferroelectric oxides have attracted increasingly intensive research both for fundamental and application issues. The physical properties of these film systems depend strongly on the particular microstructure and configuration of lattice defects. By means of an aberration corrector in a high-resolution transmission electron microscope the value of the spherical aberration CS can be tuned to negative values resulting in a novel imaging technique: The negative CS imaging (NCSI) technique. The images obtained with the NCSI technique are superior to positive CS images in the magnitude of the contrast and the image intensity of atom columns. The image signal obtained with the NCSI technique is significantly more robust against noise, resulting in measurement of atomic positions with a precision of a few picometres. In this talk, we present the results of a study using NCSI technique of the epitaxial thin-film system of PbZr0.2Ti0.8O3. The positions of all the atomic species are measured, unit cell by unit cell, with a precision of a few picometres. On this basis the relative ion displacement and the electric dipole moment for the individual unit cells are calculated. The resulting dipole moments depict the details of polarization domains, domain walls, as well as the local variation of spontaneous polarization at defect areas. C  Wa   '   N        0nn  B I01 &SN'Yf[irtf[bQZ`irtNPgeirt@b ' ,  <3fQ"`1 3 ,/events/icmp10f.xml,-, 0(J  S ~rkrk ԔԔ8c8c?C#* QZ`irt-SN'Yf[[W2 'X'X ,  T@?\O ?"6?@`NNN?Nk% \>%fg WNt]!hckؚRs\5uP[>f_\vt]fWO'`/fSNufؚvPl^ X:_ؚR5uP[>f_PvOS:_^ N cؚ[ϑRgv|^0PRNt]bPb/g (WSP[:\^[ϑ0Wh_NBaTiO3111 j[vfLub-Nv'l:w0(u[ϑؚR5uP[>f_/g[5u'lSir-NvLub0:wSvQ[~s|SN~s|:SW5u'`vq_TۏLNSP[:\^0WxvzRg [sNKmϑh_USހ5uvPgwS~s|:S 5u'`0 4$ 3"; 0nnH  0+nF ? 33___PPT10i.JPx+D=' = @B +rg#"C#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖ"D[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dd 0pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#    0 0 m(  T  C ,AIMG_4419m5%4  Zjpp9?g  2010t^,{26g  '($|  Bm?G Ve11g18efgV 15:00 16:40 0WpSN'Yf[irt'Y|i-N212Ye[,,'-d B  H{?Jp#  \Characterization at picometres precision of structure and properties of ferroelectric oxides]]-.   >    <3fQ"`2#$3 Photograph by Xiaodong Hu,  Hć3s?"`r $& *>%fg Yec _VN)R ^xvz-N_Forschungszentrum Jlich GmbH)xvzXT [N'Yf[VE5uN(xvz-N_Yec.E&B>&(P    F  <܋- / HT|N: O'YOYec emaildpyu@pku.edu.cn .%#g$-@(  BL\O"`&$<( bAbstract: Epitaxial thin films of ferroelectric oxides have attracted increasingly intensive research both for fundamental and application issues. The physical properties of these film systems depend strongly on the particular microstructure and configuration of lattice defects. By means of an aberration corrector in a high-resolution transmission electron microscope the value of the spherical aberration CS can be tuned to negative values resulting in a novel imaging technique: The negative CS imaging (NCSI) technique. The images obtained with the NCSI technique are superior to positive CS images in the magnitude of the contrast and the image intensity of atom columns. The image signal obtained with the NCSI technique is significantly more robust against noise, resulting in measurement of atomic positions with a precision of a few picometres. In this talk, we present the results of a study using NCSI technique of the epitaxial thin-film system of PbZr0.2Ti0.8O3. The positions of all the atomic species are measured, unit cell by unit cell, with a precision of a few picometres. On this basis the relative ion displacement and the electric dipole moment for the individual unit cells are calculated. The resulting dipole moments depict the details of polarization domains, domain walls, as well as the local variation of spontaneous polarization at defect areas. C  Wa   '   N        0nn  B I01 &SN'Yf[irtf[bQZ`irtNPgeirt@b ' ,  <3fQ"`1 3 ,/events/icmp10f.xml,-, 0(J  S ~rkrk ԔԔ8c8c?C#* QZ`irt-SN'Yf[[W2 'X'X ,  T@?\O ?"6?@`NNN?NM% \>%fg WNt]!hckؚRs\5uP[>f_\vt]fWO'`/fSNufؚvPl^ X:_ؚR5uP[>f_PvOS:_^ N cؚ[ϑRgv|^0PRNt]bPb/g (WSP[:\^[ϑ0Wh_NBaTiO3111 j[vfLub-Nv'l:w0(u[ϑؚR5uP[>f_/g[5u'lSir-NvLub0:wSvQ[~s|SN~s|:SW5u'`vq_TۏLNSP[:\^0WxvzRg [sNKmϑh_USހ5uvPgwS~s|:S 5u'`0 4$ 3"; 0nnH  0+nF ? 33___PPT10i.JPx+D=' = @B +r,#1#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖ"D[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dd 0pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#    0 0 u(  T  C ,AIMG_4419m5%4  Zjpp9?g  2010t^,{26g  '($|  Bm?G Ve11g18efgV 15:00 16:40 0WpSN'Yf[irt'Y|i-N212Ye[,,'-d B  H{?Jp#  \Characterization at picometres precision of structure and properties of ferroelectric oxides]]-.   >    <3fQ"`2#$3 Photograph by Xiaodong Hu,  Hć3s?"`r $& 2>%fg Yec _VN)R ^xvz-N_(Forschungszentrum Jlich GmbH)xvzXT [N'Yf[VE5uN(xvz-N_Yec.E&B>&(X    F  <܋- / HT|N: O'YOYec emaildpyu@pku.edu.cn .%#g$-@(  BL\O"`&$<( bAbstract: Epitaxial thin films of ferroelectric oxides have attracted increasingly intensive research both for fundamental and application issues. The physical properties of these film systems depend strongly on the particular microstructure and configuration of lattice defects. By means of an aberration corrector in a high-resolution transmission electron microscope the value of the spherical aberration CS can be tuned to negative values resulting in a novel imaging technique: The negative CS imaging (NCSI) technique. The images obtained with the NCSI technique are superior to positive CS images in the magnitude of the contrast and the image intensity of atom columns. The image signal obtained with the NCSI technique is significantly more robust against noise, resulting in measurement of atomic positions with a precision of a few picometres. In this talk, we present the results of a study using NCSI technique of the epitaxial thin-film system of PbZr0.2Ti0.8O3. The positions of all the atomic species are measured, unit cell by unit cell, with a precision of a few picometres. On this basis the relative ion displacement and the electric dipole moment for the individual unit cells are calculated. The resulting dipole moments depict the details of polarization domains, domain walls, as well as the local variation of spontaneous polarization at defect areas. C  Wa   '   N        0nn  B I01 &SN'Yf[irtf[bQZ`irtNPgeirt@b ' ,  <3fQ"`1 3 ,/events/icmp10f.xml,-, 0(J  S ~rkrk ԔԔ8c8c?C#* QZ`irt-SN'Yf[[W2 'X'X ,  T@?\O ?"6?@`NNN?NM% \>%fg WNt]!hckؚRs\5uP[>f_\vt]fWO'`/fSNufؚvPl^ X:_ؚR5uP[>f_PvOS:_^ N cؚ[ϑRgv|^0PRNt]bPb/g (WSP[:\^[ϑ0Wh_NBaTiO3111 j[vfLub-Nv'l:w0(u[ϑؚR5uP[>f_/g[5u'lSir-NvLub0:wSvQ[~s|SN~s|:SW5u'`vq_TۏLNSP[:\^0WxvzRg [sNKmϑh_USހ5uvPgwS~s|:S 5u'`0 4$ 3"; 0nnH  0+nF ? 33___PPT10i.JPx+D=' = @B +r1#91R#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖ"D[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0     D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dd 0pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#  rRRyZ#1(6%4 ,/ 0`DArial'YW[&{Ɩ0TTwܖ 0ܖD[SOal'YW[&{Ɩ0TTwܖ 0ܖ DўSOal'YW[&{Ɩ0TTwܖ 0ܖ0D[SO-eck'YW[&{Ɩ0TTwܖ 0ܖA@DNSe-N['YW[&{Ɩ0TTwܖ 0ܖPDfN['YW[&{Ɩ0TTwܖ 0ܖ1`DNSe~ў'YW[&{Ɩ0TTwܖ 0ܖpD|^Wў'YW[&{Ɩ0TTwܖ 0ܖ1 B-.  @n?" dd@  @@`` ( @'5& /X$R$H)A^!X?j< 0AA ff333f@f3w ʚ;d7ʚ;g42d2dd 0pPp<4dddd w 0Tw <4!d!d x 0T80___PPT10 pp?  %X#    0 0 q(  T  C ,AIMG_4419m5%4  Zxkpp9?g  2010t^,{26g  '($z  B0m?G Te12g9efgV 15:00 16:40 0WpSN'Yf[irt'Y|i-N212Ye[++'-d B  Hg?Jp#  \Characterization at picometres precision of structure and properties of ferroelectric oxides]]-.   >    <3fQ"`2#$3 Photograph by Xiaodong Hu,  HL3s?"`r $& 2>%fg Yec _VN)R ^xvz-N_(Forschungszentrum Jlich GmbH)xvzXT [N'Yf[VE5uN(xvz-N_Yec.E&B>&(X    F  <- / HT|N: O'YOYec emaildpyu@pku.edu.cn .%#g$-@&  B\O"`&$<( bAbstract: Epitaxial thin films of ferroelectric oxides have attracted increasingly intensive research both for fundamental and application issues. The physical properties of these film systems depend strongly on the particular microstructure and configuration of lattice defects. By means of an aberration corrector in a high-resolution transmission electron microscope the value of the spherical aberration CS can be tuned to negative values resulting in a novel imaging technique: The negative CS imaging (NCSI) technique. The images obtained with the NCSI technique are superior to positive CS images in the magnitude of the contrast and the image intensity of atom columns. The image signal obtained with the NCSI technique is significantly more robust against noise, resulting in measurement of atomic positions with a precision of a few picometres. In this talk, we present the results of a study using NCSI technique of the epitaxial thin-film system of PbZr0.2Ti0.8O3. The positions of all the atomic species are measured, unit cell by unit cell, with a precision of a few picometres. On this basis the relative ion displacement and the electric dipole moment for the individual unit cells are calculated. The resulting dipole moments depict the details of polarization domains, domain walls, as well as the local variation of spontaneous polarization at defect areas. 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